His father struggled to gather funds for their education. He studied in a "hut school" till fourth standard, and later did his schooling at Khrist Raja High School, Bettiah. He completed his 12th class from Maharani Janaki Kunwar College in Bettiah.
Bajpayee was married to a girl from Delhi, but got divorced during his period of struggle. He met actress Shabana Raza, who is also known as Neha, right after her debut film Kareeb (1998). The couple married in 2006 and they have a daughter.
Director Ram Gopal Varma considers him to be "an education" for himself and said he is "simply the best actor I've ever worked with." Shekhar Kapur, who directed him in Bandit Queen, recalls: "Manoj had the ability to portray a lot just by doing little. He never tried to overplay a scene and seemed totally comfortable with a minimalist statement." According to director Hansal Mehta, Manoj "has the ability to transform himself like few others."
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